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Anisotropic 2D van der Waals Magnets Hosting 1D Spin Chains

Park, Eugene
Autor Park, Eugene ORCID Department of Materials Science and Engineering, Massachusetts Institute of Technology, Cambridge, MA, 02139, USA
Philbin, John P
Autor Philbin, John P College of Letters and Science, University of California, Los Angeles, CA, 90095, USA
Chi, Hang
Autor Chi, Hang Francis Bitter Magnet Laboratory, Plasma Science and Fusion Center, Massachusetts Institute of Technology, Cambridge, MA, 02139, USA Department of Physics, University of Ottawa, Ottawa, ON, K1N 6N5, Canada Nexus for Quantum Technologies, University of Ottawa, Ottawa, ON, K1N 6N5, Canada
Sanchez, Joshua J
Autor Sanchez, Joshua J Department of Physics, Massachusetts Institute of Technology, Cambridge, MA, 02139, USA
Occhialini, Connor
Autor Occhialini, Connor Department of Physics, Massachusetts Institute of Technology, Cambridge, MA, 02139, USA
Varnavides, Georgios
Autor Varnavides, Georgios Miller Institute for Basic Research in Science, University of California, Berkeley, CA, 94720, USA National Center for Electron Microscopy, Molecular Foundry, Lawrence Berkeley National Laboratory, Berkeley, CA, 94720, USA
Curtis, Jonathan B
Autor Curtis, Jonathan B College of Letters and Science, University of California, Los Angeles, CA, 90095, USA
Song, Zhigang
Autor Song, Zhigang John A. Paulson School of Engineering and Applied Sciences, Harvard University, Cambridge, MA, 02139, USA
Klein, Julian
Autor Klein, Julian Department of Materials Science and Engineering, Massachusetts Institute of Technology, Cambridge, MA, 02139, USA
Thomsen, Joachim D
Autor Thomsen, Joachim D Department of Materials Science and Engineering, Massachusetts Institute of Technology, Cambridge, MA, 02139, USA College of Letters and Science, University of California, Los Angeles, CA, 90095, USA
Han, Myung-Geun
Autor Han, Myung-Geun Condensed Matter Physics and Materials Science Department, Brookhaven National Laboratory, Upton, NY, 11973, USA
Foucher, Alexandre C
Autor Foucher, Alexandre C Department of Materials Science and Engineering, Massachusetts Institute of Technology, Cambridge, MA, 02139, USA
Mosina, Kseniia
Autor Mosina, Kseniia Department of Inorganic Chemistry, University of Chemistry and Technology Prague, Technická 5, Prague, 166 28, Czech Republic
Kumawat, Deepika
Autor Kumawat, Deepika Department of Physics, Massachusetts Institute of Technology, Cambridge, MA, 02139, USA Department of Physics, Mount Holyoke College, South Hadley, MA, 01075, USA
Gonzalez-Yepez, N
Autor Gonzalez-Yepez, N Department of Physics, Massachusetts Institute of Technology, Cambridge, MA, 02139, USA
Zhu, Yimei
Autor Zhu, Yimei Condensed Matter Physics and Materials Science Department, Brookhaven National Laboratory, Upton, NY, 11973, USA
Sofer, Zdeněk
Autor Sofer, Zdeněk Department of Inorganic Chemistry, University of Chemistry and Technology Prague, Technická 5, Prague, 166 28, Czech Republic
Comin, Riccardo
Autor Comin, Riccardo Department of Physics, Massachusetts Institute of Technology, Cambridge, MA, 02139, USA
Moodera, Jagadeesh S
Autor Moodera, Jagadeesh S Francis Bitter Magnet Laboratory, Plasma Science and Fusion Center, Massachusetts Institute of Technology, Cambridge, MA, 02139, USA Department of Physics, Massachusetts Institute of Technology, Cambridge, MA, 02139, USA
Narang, Prineha
Autor Narang, Prineha College of Letters and Science, University of California, Los Angeles, CA, 90095, USA
Ross, Frances M
Autor Ross, Frances M ORCID Department of Materials Science and Engineering, Massachusetts Institute of Technology, Cambridge, MA, 02139, USA

Advanced materials (Deerfield Beach, Fla.). 2024 Aug ; 36 (31) : e2401534. [epub] 20240603

Adv Mater
ISSN 1521-4095 | 0935-9648
Zdroj

Status PubMed-not-MEDLINE Jazyk nizozemština (holandština) Země Německo Médium print-electronic

Typ dokumentu anglický abstrakt, časopisecké články

Perzistentní odkaz https://www.medvik.cz/link/pmid38795019

Grantová podpora
Canada Research Chairs
RGPIN-2024-06497 Natural Sciences and Engineering Research Council of Canada
2138167 National Science Foundation MPS-Ascend Postdoctoral Research Fellowship
LL2101 ERC-CZ program
Ministry of Education Youth and Sports
N00014-20-1-2306 Office of Naval Research
W911NF-20-1-0074 Army Research Office
W911NF-20-2-0061 Army Research Office
NSF-DMR 2218550 National Science Foundation
NSF-DMR 1231319 National Science Foundation
NSF-ECCS-1944085 National Science Foundation
W911NF1810432 Multidisciplinary University Research Initiative
GBMF8048 Gordon and Betty Moore Foundation
DE-SC0012704 U.S. Department of Energy
DE-SC0022277 U.S. Department of Energy
W911NF-19-2-0015 Army Research Laboratory
MathWorks

Odkazy
PubMed 38795019
DOI 10.1002/adma.202401534
Knihovny.cz E-zdroje

Klíčová slova
1D magnetism, 2D magnets, 2D materials, scanning transmission electron microscopy,
Publikační typ
anglický abstrakt MeSH
časopisecké články MeSH

The exploration of 1D magnetism, frequently portrayed as spin chains, constitutes an actively pursued research field that illuminates fundamental principles in many-body problems and applications in magnonics and spintronics. The inherent reduction in dimensionality often leads to robust spin fluctuations, impacting magnetic ordering and resulting in novel magnetic phenomena. Here, structural, magnetic, and optical properties of highly anisotropic 2D van der Waals antiferromagnets that uniquely host spin chains are explored. First-principle calculations reveal that the weakest interaction is interchain, leading to essentially 1D magnetic behavior in each layer. With the additional degree of freedom arising from its anisotropic structure, the structure is engineered by alloying, varying the 1D spin chain lengths using electron beam irradiation, or twisting for localized patterning, and spin textures are calculated, predicting robust stability of the antiferromagnetic ordering. Comparing with other spin chain magnets, these materials are anticipated to bring fresh perspectives on harvesting low-dimensional magnetism.

College of Letters and Science University of California Los Angeles CA 90095 USA

Condensed Matter Physics and Materials Science Department Brookhaven National Laboratory Upton NY 11973 USA

Department of Inorganic Chemistry University of Chemistry and Technology Prague Technická 5 Prague 166 28 Czech Republic

Department of Materials Science and Engineering Massachusetts Institute of Technology Cambridge MA 02139 USA

Department of Physics Massachusetts Institute of Technology Cambridge MA 02139 USA

Department of Physics Mount Holyoke College South Hadley MA 01075 USA

Department of Physics University of Ottawa Ottawa ON K1N 6N5 Canada

Francis Bitter Magnet Laboratory Plasma Science and Fusion Center Massachusetts Institute of Technology Cambridge MA 02139 USA

John A Paulson School of Engineering and Applied Sciences Harvard University Cambridge MA 02139 USA

Miller Institute for Basic Research in Science University of California Berkeley CA 94720 USA

National Center for Electron Microscopy Molecular Foundry Lawrence Berkeley National Laboratory Berkeley CA 94720 USA

Nexus for Quantum Technologies University of Ottawa Ottawa ON K1N 6N5 Canada

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