Anisotropic 2D van der Waals Magnets Hosting 1D Spin Chains
Status PubMed-not-MEDLINE Jazyk nizozemština (holandština) Země Německo Médium print-electronic
Typ dokumentu anglický abstrakt, časopisecké články
Grantová podpora
Canada Research Chairs
RGPIN-2024-06497
Natural Sciences and Engineering Research Council of Canada
2138167
National Science Foundation MPS-Ascend Postdoctoral Research Fellowship
LL2101
ERC-CZ program
Ministry of Education Youth and Sports
N00014-20-1-2306
Office of Naval Research
W911NF-20-1-0074
Army Research Office
W911NF-20-2-0061
Army Research Office
NSF-DMR 2218550
National Science Foundation
NSF-DMR 1231319
National Science Foundation
NSF-ECCS-1944085
National Science Foundation
W911NF1810432
Multidisciplinary University Research Initiative
GBMF8048
Gordon and Betty Moore Foundation
DE-SC0012704
U.S. Department of Energy
DE-SC0022277
U.S. Department of Energy
W911NF-19-2-0015
Army Research Laboratory
MathWorks
Odkazy
PubMed
38795019
DOI
10.1002/adma.202401534
Knihovny.cz E-zdroje
- Klíčová slova
- 1D magnetism, 2D magnets, 2D materials, scanning transmission electron microscopy,
- Publikační typ
- anglický abstrakt MeSH
- časopisecké články MeSH
The exploration of 1D magnetism, frequently portrayed as spin chains, constitutes an actively pursued research field that illuminates fundamental principles in many-body problems and applications in magnonics and spintronics. The inherent reduction in dimensionality often leads to robust spin fluctuations, impacting magnetic ordering and resulting in novel magnetic phenomena. Here, structural, magnetic, and optical properties of highly anisotropic 2D van der Waals antiferromagnets that uniquely host spin chains are explored. First-principle calculations reveal that the weakest interaction is interchain, leading to essentially 1D magnetic behavior in each layer. With the additional degree of freedom arising from its anisotropic structure, the structure is engineered by alloying, varying the 1D spin chain lengths using electron beam irradiation, or twisting for localized patterning, and spin textures are calculated, predicting robust stability of the antiferromagnetic ordering. Comparing with other spin chain magnets, these materials are anticipated to bring fresh perspectives on harvesting low-dimensional magnetism.
College of Letters and Science University of California Los Angeles CA 90095 USA
Department of Physics Massachusetts Institute of Technology Cambridge MA 02139 USA
Department of Physics Mount Holyoke College South Hadley MA 01075 USA
Department of Physics University of Ottawa Ottawa ON K1N 6N5 Canada
John A Paulson School of Engineering and Applied Sciences Harvard University Cambridge MA 02139 USA
Miller Institute for Basic Research in Science University of California Berkeley CA 94720 USA
Nexus for Quantum Technologies University of Ottawa Ottawa ON K1N 6N5 Canada
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