Strain Regulating and Kinetics Accelerating of Micro-Sized Silicon Anodes via Dual-Size Hollow Graphitic Carbons Conductive Additives
Status PubMed-not-MEDLINE Jazyk angličtina Země Německo Médium print-electronic
Typ dokumentu časopisecké články
Grantová podpora
52071225
National Natural Science Foundation of China
51672181
National Natural Science Foundation of China
CZ.02.1.01/0.0/0.0/16_019/0000853
Institute of Environmental Technology -Excellent Research
GZ 1400
Sino-German Research Institute
PubMed
36433825
DOI
10.1002/smll.202205284
Knihovny.cz E-zdroje
- Klíčová slova
- dual-size conductive additives, hollow graphitic carbons, kinetics accelerating, micro-sized Si anodes, strain regulating,
- Publikační typ
- časopisecké články MeSH
Micro-sized silicon (µSi) anode features fewer interfacial side reactions and lower costs compared to nanosized silicon, and has higher commercial value when applied as a lithium-ion battery (LIB) anode. However, the high localized stress generated during (de)lithiation causes electrode breakdown and performance deterioration of the µSi anode. In this work, hollow graphitic carbons with tailored dual sizes are employed as conductive additives for the µSi anode to overcome electrode failure. The dual-size hollow graphitic carbons (HGC) additives consist of particles with micrometer size similar to the µSi particles; these additives are used for strain regulation. Additionally, nanometer-size particles similar to commercial carbon black Spheron (SP) are used mainly for kinetics acceleration. In addition to building an efficient conductive network, the dual-size hollow graphitic carbon conductive additive prevents the fracture of the electrode by reducing local stress and alleviating volume expansion. The µSi anode with dual-size hollow graphitic carbons as conductive additives achieves an impressive capacity of 651.4 mAh g-1 after 500 cycles at a high current density of 2 A g-1 . These findings suggest that dual-size hollow graphitic carbons are expected to be superior conductive additives for micro-sized alloy anodes similar to µSi.
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