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Ultrafast Formation of Charge Transfer Trions at Molecular-Functionalized 2D MoS2 Interfaces

Jing, Yuancheng
Autor Jing, Yuancheng ORCID Department of Chemistry and Biochemistry, University of California, San Diego, 9500 Gilman Drive, MC 0358, La Jolla, California, 92093-0358, United States
Liang, Kangkai
Autor Liang, Kangkai Material Science and Engineering Program, University of California, San Diego, 9500 Gilman Drive, MC 0418, La Jolla, California, 92093-0418, United States
Muir, Nicole S
Autor Muir, Nicole S Department of Chemistry and Biochemistry, University of California, San Diego, 9500 Gilman Drive, MC 0358, La Jolla, California, 92093-0358, United States
Zhou, Hao
Autor Zhou, Hao Material Science and Engineering Program, University of California, San Diego, 9500 Gilman Drive, MC 0418, La Jolla, California, 92093-0418, United States
Li, Zhehao
Autor Li, Zhehao Material Science and Engineering Program, University of California, San Diego, 9500 Gilman Drive, MC 0418, La Jolla, California, 92093-0418, United States
Palasz, Joseph M
Autor Palasz, Joseph M ORCID Department of Chemistry and Biochemistry, University of California, San Diego, 9500 Gilman Drive, MC 0358, La Jolla, California, 92093-0358, United States
Sorbie, Jonathan
Autor Sorbie, Jonathan Department of Chemistry and Biochemistry, University of California, San Diego, 9500 Gilman Drive, MC 0358, La Jolla, California, 92093-0358, United States
Wang, Chenglai
Autor Wang, Chenglai ORCID Department of Chemistry and Biochemistry, University of California, San Diego, 9500 Gilman Drive, MC 0358, La Jolla, California, 92093-0358, United States
Cushing, Scott K
Autor Cushing, Scott K ORCID Division of Chemistry and Chemical Engineering, California Institute of Technology, 1200 E California Blvd, MC 127-72, Pasadena, California, 91125, United States
Kubiak, Clifford P
Autor Kubiak, Clifford P ORCID Department of Chemistry and Biochemistry, University of California, San Diego, 9500 Gilman Drive, MC 0358, La Jolla, California, 92093-0358, United States
Sofer, Zdeněk
Autor Sofer, Zdeněk Department of Inorganic Chemistry, University of Chemistry and Technology, Prague, Technická 5, 166 28, Prague 6, Czech Republic
Li, Shaowei
Autor Li, Shaowei ORCID Department of Chemistry and Biochemistry, University of California, San Diego, 9500 Gilman Drive, MC 0358, La Jolla, California, 92093-0358, United States Material Science and Engineering Program, University of California, San Diego, 9500 Gilman Drive, MC 0418, La Jolla, California, 92093-0418, United States
Xiong, Wei
Autor Xiong, Wei ORCID Department of Chemistry and Biochemistry, University of California, San Diego, 9500 Gilman Drive, MC 0358, La Jolla, California, 92093-0358, United States Material Science and Engineering Program, University of California, San Diego, 9500 Gilman Drive, MC 0418, La Jolla, California, 92093-0418, United States

Angewandte Chemie (International ed. in English). 2024 Jul 22 ; 63 (30) : e202405123. [epub] 20240619

Angew Chem Int Ed Engl
ISSN 1521-3773 | 1433-7851
Zdroj

Status PubMed-not-MEDLINE Jazyk angličtina Země Německo Médium print-electronic

Typ dokumentu časopisecké články

Perzistentní odkaz https://www.medvik.cz/link/pmid38714495

Grantová podpora
DE-FOA-0002449 U.S. Department of Energy
CHE-2303936 National Science Foundation
CHE-2153757 National Science Foundation
project LL2101 Ministry of Education Youth and Sports (MEYS) ERC-CZ program
reg. No. CZ.02.1.01/0.0/0.0/15_003/0000444 Project Advanced Functional Nanorobots
DE-FOA-0002449 Office of Science

PubMed 38714495
DOI 10.1002/anie.202405123
Knihovny.cz E-zdroje

Klíčová slova
Time-resolved interfacial-sensitive spectroscopy, charge transfer, molecular- functionalized monolayer TMD, sum frequency generation, trion,
Publikační typ
časopisecké články MeSH

In this work, we investigate trion dynamics occurring at the heterojunction between organometallic molecules and a monolayer transition metal dichalcogenide (TMD) with transient electronic sum frequency generation (tr-ESFG) spectroscopy. By pumping at 2.4 eV with laser pulses, we have observed an ultrafast hole transfer, succeeded by the emergence of charge-transfer trions. This observation is facilitated by the cancellation of ground state bleach and stimulated emission signals due to their opposite phases, making tr-ESFG especially sensitive to the trion formation dynamics. The presence of charge-transfer trion at molecular functionalized TMD monolayers suggests the potential for engineering the local electronic structures and dynamics of specific locations on TMDs and offers a potential for transferring unique electronic attributes of TMD to the molecular layers.

Department of Chemistry and Biochemistry University of California San Diego 9500 Gilman Drive MC 0358 La Jolla California 92093 0358 United States

Department of Inorganic Chemistry University of Chemistry and Technology Prague Technická 5 166 28 Prague 6 Czech Republic

Division of Chemistry and Chemical Engineering California Institute of Technology 1200 E California Blvd MC 127 72 Pasadena California 91125 United States

Material Science and Engineering Program University of California San Diego 9500 Gilman Drive MC 0418 La Jolla California 92093 0418 United States

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Ultrafast Formation of Charge Transfer Trions at Molecular-Functionalized 2D MoS2 Interfaces

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