Mn-Rich MnSb2 Te4 : A Topological Insulator with Magnetic Gap Closing at High Curie Temperatures of 45-50 K
Status PubMed-not-MEDLINE Jazyk angličtina Země Německo Médium print-electronic
Typ dokumentu časopisecké články
Grantová podpora
I 4493
Austrian Science Fund FWF - Austria
P 30960
Austrian Science Fund FWF - Austria
PubMed
34469013
PubMed Central
PMC11468489
DOI
10.1002/adma.202102935
Knihovny.cz E-zdroje
- Klíčová slova
- Mn-Sb site exchange, MnSb 2Te 4, magnetic bandgap, magnetic topological insulators, magnetization, molecular beam epitaxy,
- Publikační typ
- časopisecké články MeSH
Ferromagnetic topological insulators exhibit the quantum anomalous Hall effect, which is potentially useful for high-precision metrology, edge channel spintronics, and topological qubits. The stable 2+ state of Mn enables intrinsic magnetic topological insulators. MnBi2 Te4 is, however, antiferromagnetic with 25 K Néel temperature and is strongly n-doped. In this work, p-type MnSb2 Te4 , previously considered topologically trivial, is shown to be a ferromagnetic topological insulator for a few percent Mn excess. i) Ferromagnetic hysteresis with record Curie temperature of 45-50 K, ii) out-of-plane magnetic anisotropy, iii) a 2D Dirac cone with the Dirac point close to the Fermi level, iv) out-of-plane spin polarization as revealed by photoelectron spectroscopy, and v) a magnetically induced bandgap closing at the Curie temperature, demonstrated by scanning tunneling spectroscopy (STS), are shown. Moreover, a critical exponent of the magnetization β ≈ 1 is found, indicating the vicinity of a quantum critical point. Ab initio calculations reveal that Mn-Sb site exchange provides the ferromagnetic interlayer coupling and the slight excess of Mn nearly doubles the Curie temperature. Remaining deviations from the ferromagnetic order open the inverted bulk bandgap and render MnSb2 Te4 a robust topological insulator and new benchmark for magnetic topological insulators.
2 Institute of Physics B and JARA FIT RWTH Aachen Unversity 52074 Aachen Germany
Centro de Física de Materiales Centro Mixto CSIC UPV EHU San Sebastián Donostia 20018 Spain
Department of Condensed Matter Physics Masaryk University Kotlářská 267 2 Brno 61137 Czech Republic
Department of Physics and Astronomy Universitet Uppsala Lägerhyddsvägen 1 Uppsala 75120 Sweden
Donostia International Physics Center San Sebastián Donostia 20018 Spain
Helmholtz Zentrum Berlin für Materialien und Energie Albert Einstein Straße 15 12489 Berlin Germany
IKERBASQUE Basque Foundation for Science Bilbao 48011 Spain
Max Planck Institute of Microstructure Physics Weinberg 2 06120 Halle Germany
Saint Petersburg State University Saint Petersburg 198504 Russia
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