Selected ice nanoparticle accelerator hypervelocity impact mass spectrometer (SELINA-HIMS): features and impacts of charged particles
Status PubMed-not-MEDLINE Jazyk angličtina Země Velká Británie, Anglie Médium print-electronic
Typ dokumentu časopisecké články
Grantová podpora
AB 63/25-1
Deutsche Forschungsgemeinschaft
21-11931J
Grantová Agentura České Republiky
PubMed
38736336
DOI
10.1098/rsta.2023.0208
Knihovny.cz E-zdroje
- Klíčová slova
- analogue experiments, hypervelocity, ice accelerator, ice particles, impact,
- Publikační typ
- časopisecké články MeSH
The selected ice nanoparticle accelerator, SELINA, was used to prepare beams of single ice particles with positive or negative charge. Positively charged particles were prepared from deionized water and 0.05-0.2 molar solutions of sodium chloride in water, and negatively charged ice particles were generated from water without salt. Depending on the electrospray source configuration, the measured particles vary from 50 to 1000 nm in diameter. The kinetic energy per charge for all particles was set to 200 eV by the collisional equilibration in quadrupoles, which resulted in primary velocities up to 600 m/s for the lowest m/z particles. The electrospray ionization and thus particle formation from SELINA become less efficient with increasing salt concentration, resulting in a lower detected particle frequency and size. Good instrument operation is achievable for concentrations below 0.2 M. After we have verified and characterized positively and negatively charged ice particles, we have combined SELINA with a target and time-of-flight spectrometer for a 'proof-of-principle' post acceleration of 120 nm particles towards hypervelocity (v ~ 3000 m/s) and detection of fragments from the particle impact (SELINA-HIMS). General conditions are discussed for the acceleration of particles between 50 and 1000 nm to velocities well above 3000 m/s with SELINA-HIMS instrument. This article is part of the theme issue 'Dust in the Solar System and beyond'.
Institute of Geological Sciences Freie Universität Berlin Berlin 12249 Germany
J Heyrovský Institute of Physical Chemistry of the Czech Academy of Sciences Prague 18223 Czechia
Laboratory for Atmospheric and Space Physics University of Colorado Boulder CO 80303 USA
Leibniz Institute of Surface Engineering Leipzig 04318 Germany
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