1D Coordination π-d Conjugated Polymers with Distinct Structures Defined by the Choice of the Transition Metal: Towards a New Class of Antiaromatic Macrocycles
Status PubMed-not-MEDLINE Jazyk angličtina Země Německo Médium print-electronic
Typ dokumentu časopisecké články
Grantová podpora
20-13692X
Grantová Agentura České Republiky
LM2018110, CZ.02.1.01/0.0/0.0/16_019/0000754
Ministerstvo Školství, Mládeže a Tělovýchovy
PubMed
32886405
DOI
10.1002/anie.202011462
Knihovny.cz E-zdroje
- Klíčová slova
- coordination polymers, macrocycles, on-surface synthesis, scanning probe microscopy, π-d conjugation,
- Publikační typ
- časopisecké články MeSH
Recently π-d conjugated coordination polymers have received a lot of attention owing to their unique material properties, although synthesis of long and defect-free polymers remains challenging. Herein we introduce a novel on-surface synthesis of coordination polymers with quinoidal ligands under ultra-high vacuum conditions, which enables formation of flexible coordination polymers with lengths up to hundreds of nanometers. Moreover, this procedure allows the incorporation of different transition-metal atoms with four- or two-fold coordination. Remarkably, the two-fold coordination mode revealed the formation of wires constituted by (electronically) independent 12-membered antiaromatic macrocycles linked together through two C-C single bonds.
Aix Marseille Université CINaM UMR 7325 CNRS Campus de Luminy 13288 Marseille cedex 09 France
Institute of Physics Czech Academy of Sciences Cukrovarnická 10 16200 Prague Czech Republic
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Light-Controlled Multiconfigurational Conductance Switching in a Single 1D Metal-Organic Wire
