Stable and Highly Active Single Atom Configurations for Photocatalytic H2 Generation

. 2024 Jun ; 36 (25) : e2400626. [epub] 20240404

Status PubMed-not-MEDLINE Jazyk angličtina Země Německo Médium print-electronic

Typ dokumentu časopisecké články

Perzistentní odkaz   https://www.medvik.cz/link/pmid38520245

Grantová podpora
CZ.02.1.01/0.0/0.0/15_003/0000416 European Regional Development Fund
Ministry of Education, Youth and Sports of the Czech Republic
Deutsche Forschungsgemeinschaft
HORIZON-WIDERA-2021-ACCESS-03-01 European Union's Horizon 2020 project SAN4Fuel
101079384 European Union's Horizon 2020 project SAN4Fuel
23-08019X Czech Science Foundation

The employment of single atoms (SAs), especially Pt SAs, as co-catalysts in photocatalytic H2 generation has gained significant attention due to their exceptional efficiency. However, a major challenge in their application is the light-induced agglomeration of these SAs into less active nanosized particles under photocatalytic conditions. This study addresses the stability and reactivity of Pt SAs on TiO2 surfaces by investigating various post-deposition annealing treatments in air, Ar, and Ar-H2 environments at different temperatures. It is described that annealing in an Ar-H2 atmosphere optimally stabilizes SA configurations, forming stable 2D rafts of assembled SAs ≈0.5-1 nm in diameter. These rafts not only resist light-induced agglomeration but also exhibit significantly enhanced H2 production efficiency. The findings reveal a promising approach to maintaining the high reactivity of Pt SAs while overcoming the critical challenge of their stability under photocatalytic conditions.

Zobrazit více v PubMed

Y. Chen, S. Ji, C. Chen, Q. Peng, D. Wang, Y. Li, Joule 2018, 2, 1242.

H. Zhang, G. Liu, L. Shi, J. Ye, Adv. Energy Mater. 2018, 8, 1701343.

S. Mitchell, J. Pérez‐Ramírez, Nat. Commun. 2020, 11, 4302.

D. Liu, Q. He, S. Ding, L. Song, Adv. Energy Mater. 2020, 10, 2001482.

X. Li, X. Yang, Y. Huang, T. Zhang, B. Liu, Adv. Mater. 2019, 31, 1902031.

Y. Zhou, J. Li, X. Gao, W. Chu, G. Gao, L.‐W. Wang, J. Mater. Chem. A 2021, 9, 9979.

Q. Zhang, J. Guan, Adv. Funct. Mater. 2020, 30, 2000768.

C. Zhu, S. Fu, Q. Shi, D. Du, Y. Lin, Angew. Chem. 2017, 56, 13944.

J. Su, R. Ge, Y. Dong, F. Hao, L. Chen, J. Mater. Chem. A 2018, 6, 14025.

W. Zang, Z. Kou, S. J. Pennycook, J. Wang, Adv. Energy Mater. 2020, 10, 1903181.

Q. Zhang, J. Guan, Sol. RRL 2020, 4, 2000283.

Q. Wang, D. Zhang, Y. Chen, W.‐F. Fu, X.‐J. Lv, ACS Sustainable Chem. Eng. 2019, 7, 6430.

J. Fu, S. Wang, Z. Wang, K. Liu, H. Li, H. Liu, J. Hu, X. Xu, H. Li, M. Liu, Front. Phys. 2020, 15, 33201.

F. Zhang, Y. Zhu, Q. Lin, L. Zhang, X. Zhang, H. Wang, Energy Environ. Sci. 2021, 14, 2954.

X. Chen, S. Shen, L. Guo, S. S. Mao, Chem. Rev. 2010, 110, 6503.

A. J. Bard, J. Photochem. 1979, 10, 59.

S. Bai, W. Yin, L. Wang, Z. Li, Y. Xiong, RSC Adv. 2016, 6, 57446.

K. G. Pickup, B. M. W. Trapnell, J. Chem. Phys. 1956, 25, 182.

S. Katz, G. B. Kistiakowsky, R. F. Steiner, J. Am. Chem. Soc. 1949, 71, 2258.

W. V. Smith, J. Chem. Phys. 1943, 11, 110.

J. Schneider, M. Matsuoka, M. Takeuchi, J. Zhang, Y. Horiuchi, M. Anpo, D. W. Bahnemann, Chem. Rev. 2014, 114, 9919.

C. Dong, C. Lian, S. Hu, Z. Deng, J. Gong, M. Li, H. Liu, M. Xing, J. Zhang, Nat. Commun. 2018, 9, 1252.

J. Ma, X. Tan, Q. Zhang, Y. Wang, J. Zhang, L. Wang, ACS Catal. 2021, 11, 3352.

Y. Ben‐Shahar, F. Scotognella, I. Kriegel, L. Moretti, G. Cerullo, E. Rabani, U. Banin, Nat. Commun. 2016, 7, 10413.

F. Xue, C. Chen, W. Fu, M. Liu, C. Liu, P. Guo, S. Shen, J. Phys. Chem. C 2018, 122, 25165.

C. Dessal, L. Martínez, C. Maheu, T. Len, F. Morfin, J. L. Rousset, E. Puzenat, P. Afanasiev, M. Aouine, L. Soler, J. Llorca, L. Piccolo, J. Catal. 2019, 375, 155.

D. Riassetto, C. Holtzinger, M. Langlet, J. Mater. Sci. 2009, 44, 2637.

I. Vamvasakis, B. Liu, G. S. Armatas, Adv. Funct. Mater. 2016, 26, 8062.

S. Gutić, A. Dobrota, E. Fako, N. Skorodumova, N. López, I. Pašti, Catalysts 2020, 10, 290.

M. Li, K. Duanmu, C. Wan, T. Cheng, L. Zhang, S. Dai, W. Chen, Z. Zhao, P. Li, H. Fei, Y. Zhu, R. Yu, J. Luo, K. Zang, Z. Lin, M. Ding, J. Huang, H. Sun, J. Guo, X. Pan, W. A. Goddard, P. Sautet, Y. Huang, X. Duan, Nat. Catal. 2019, 2, 495.

K. Maiti, S. Maiti, M. T. Curnan, H. J. Kim, J. W. Han, Adv. Energy Mater. 2021, 11, 2101670.

S. Qin, J. Will, H. Kim, N. Denisov, S. Carl, E. Spiecker, P. Schmuki, ACS Energy Lett. 2023, 8, 1209.

D. Wang, Z.‐P. Liu, W.‐M. Yang, ACS Catal. 2018, 8, 7270.

N. Denisov, S. Qin, J. Will, B. N. Vasiljevic, N. V. Skorodumova, I. A. Pašti, B. B. Sarma, B. Osuagwu, T. Yokosawa, J. Voss, J. Wirth, E. Spiecker, P. Schmuki, Adv. Mater. 2023, 35, 2206569.

J. Xing, H. B. Jiang, J. F. Chen, Y. H. Li, L. Wu, S. Yang, L. R. Zheng, H. F. Wang, P. Hu, H. J. Zhao, H. G. Yang, J. Mater. Chem. A 2013, 1, 15258.

J. Xing, J. F. Chen, Y. H. Li, W. T. Yuan, Y. Zhou, L. R. Zheng, H. F. Wang, P. Hu, Y. Wang, H. J. Zhao, Y. Wang, H. G. Yang, Chemistry 2014, 20, 2138.

J. Cai, A. Cao, Z. Wang, S. Lu, Z. Jiang, X.‐Y. Dong, X. Li, S.‐Q. Zang, J. Mater. Chem. A 2021, 9, 13890.

Y. Chen, S. Ji, W. Sun, Y. Lei, Q. Wang, A. Li, W. Chen, G. Zhou, Z. Zhang, Y. Wang, L. Zheng, Q. Zhang, L. Gu, X. Han, D. Wang, Y. Li, Angew. Chem. 2020, 132, 1311.

S. Hejazi, S. Mohajernia, B. Osuagwu, G. Zoppellaro, P. Andryskova, O. Tomanec, S. Kment, R. Zbořil, P. Schmuki, Adv. Mater. 2020, 32, 1908505.

Q. Zuo, T. Liu, C. Chen, Y. Ji, X. Gong, Y. Mai, Y. Zhou, Angew. Chem. 2019, 58, 10198.

X. Hu, J. Song, J. Luo, H. Zhang, Z. Sun, C. Li, S. Zheng, Q. Liu, J. Energy Chem. 2021, 62, 1.

H. Hu, J. Wang, P. Tao, C. Song, W. Shang, T. Deng, J. Wu, J. Mater. Chem. A 2022, 10, 5835.

Y. Chen, Z. Huang, Z. Ma, J. Chen, X. Tang, Catal. Sci. Technol. 2017, 7, 4250.

L. Liu, D. M. Meira, R. Arenal, P. Concepcion, A. V. Puga, A. Corma, ACS Catal. 2019, 9, 10626.

J. T. Miller, M. Schreier, A. J. Kropf, J. R. Regalbuto, J. Catal. 2004, 225, 203.

J. Sun, J. Zhang, H. Fu, H. Wan, Y. Wan, X. Qu, Z. Xu, D. Yin, S. Zheng, Appl. Catal., B 2018, 229, 32.

X. Chen, X.‐B. Wang, S. Han, D. Wang, C. Li, W. Guan, W.‐Y. Li, C. Liang, ACS Appl. Mater. Interfaces 2022, 14, 590.

G. Cha, I. Hwang, S. Hejazi, A. S. Dobrota, I. A. Pašti, B. Osuagwu, H. Kim, J. Will, T. Yokosawa, Z. Badura, Š. Kment, S. Mohajernia, A. Mazare, N. V. Skorodumova, E. Spiecker, P. Schmuki, iScience 2021, 24, 102938.

G. Cha, A. Mazare, I. Hwang, N. Denisov, J. Will, T. Yokosawa, Z. Badura, G. Zoppellaro, A. B. Tesler, E. Spiecker, P. Schmuki, Electrochim. Acta 2022, 412, 140129.

S.‐M. Wu, I. Hwang, B. Osuagwu, J. Will, Z. Wu, B. B. Sarma, F.‐F. Pu, L.‐Y. Wang, Z. Badura, G. Zoppellaro, E. Spiecker, P. Schmuki, ACS Catal. 2023, 13, 33.

L. DeRita, S. Dai, K. Lopez‐Zepeda, N. Pham, G. W. Graham, X. Pan, P. Christopher, J. Am. Chem. Soc. 2017, 139, 14150.

H. V. Thang, G. Pacchioni, L. DeRita, P. Christopher, J. Catal. 2018, 367, 104.

L. Chen, R. R. Unocic, A. S. Hoffman, J. Hong, A. H. Braga, Z. Bao, S. R. Bare, J. Szanyi, JACS Au 2021, 1, 977.

X. Zhou, I. Hwang, O. Tomanec, D. Fehn, A. Mazare, R. Zboril, K. Meyer, P. Schmuki, Adv. Funct. Mater. 2021, 31, 2102843.

Z. Wu, I. Hwang, G. Cha, S. Qin, O. Tomanec, Z. Badura, S. Kment, R. Zboril, P. Schmuki, Small 2022, 18, 2104892.

Y. Wang, I. Hwang, Z. Wu, P. Schmuki, Electrochem. Commun. 2021, 133, 107166.

I. Hwang, A. Mazare, J. Will, T. Yokosawa, E. Spiecker, P. Schmuki, Adv. Funct. Mater. 2022, 32, 2207849.

S. Qin, N. Denisov, J. Will, J. Kolařík, E. Spiecker, P. Schmuki, Sol. RRL 2022, 6, 2101026.

S. Qin, N. Denisov, B. B. Sarma, I. Hwang, D. E. Doronkin, O. Tomanec, S. Kment, P. Schmuki, Adv. Mater. Interfaces 2022, 9, 2200808.

L. DeRita, J. Resasco, S. Dai, A. Boubnov, H. V. Thang, A. S. Hoffman, I. Ro, G. W. Graham, S. R. Bare, G. Pacchioni, X. Pan, P. Christopher, Nat. Mater. 2019, 18, 746.

H. Kim, Y. Wang, N. Denisov, Z. Wu, Š. Kment, P. Schmuki, J. Mater. Sci. 2022, 57, 12960.

Y. Wang, S. Qin, N. Denisov, H. Kim, Z. Bad'ura, B. B. Sarma, P. Schmuki, Adv. Mater. 2023, 35, 2211814.

L. Chang, S.‐T. Yong, S.‐P. Chai, L. K. Putri, L.‐L. Tan, A. R. Mohamed, Mater. Today Chem. 2023, 27, 101334.

J. Zhao, R. Shi, Z. Li, C. Zhou, T. Zhang, Nano Sel. 2020, 1, 12.

T. J. Lee, Y. G. Kim, J. Catal. 1984, 90, 279.

X. Zhang, Z. Li, W. Pei, G. Li, W. Liu, P. Du, Z. Wang, Z. Qin, H. Qi, X. Liu, S. Zhou, J. Zhao, B. Yang, W. Shen, ACS Catal. 2022, 12, 3634.

P. N. Plessow, F. Abild‐Pedersen, ACS Catal. 2016, 6, 7098.

Z. Tian, Y. Da, M. Wang, X. Dou, X. Cui, J. Chen, R. Jiang, S. Xi, B. Cui, Y. Luo, H. Yang, Y. Long, Y. Xiao, W. Chen, Nat. Commun. 2023, 14, 142.

H. Pan, X. Wang, Z. Xiong, M. Sun, M. Murugananthan, Y. Zhang, Environ. Res. 2021, 198, 111176.

S. Cai, L. Wang, S. Heng, H. Li, Y. Bai, D. Dang, Q. Wang, P. Zhang, C. He, J. Phys. Chem. C 2020, 124, 24566.

T.‐Y. Chang, Y. Tanaka, R. Ishikawa, K. Toyoura, K. Matsunaga, Y. Ikuhara, N. Shibata, Nano Lett. 2014, 14, 134.

Y. Zhang, Y. Wang, K. Su, F. Wang, J. Mol. Model. 2022, 28, 175.

J. Wan, W. Chen, C. Jia, L. Zheng, J. Dong, X. Zheng, Y. Wang, W. Yan, C. Chen, Q. Peng, D. Wang, Y. Li, Adv. Mater. 2018, 30, 1705369.

C. J. Powell, A. Jablonski, NIST Electron Inelastic‐Mean‐Free‐Path database ‐ version 1.2 2010, https://www.nist.gov/srd/nist‐standard‐reference‐database‐71.

K. Ding, A. Gulec, A. M. Johnson, N. M. Schweitzer, G. D. Stucky, L. D. Marks, P. C. Stair, Science 2015, 350, 189.

L. Nie, D. Mei, H. Xiong, B. Peng, Z. Ren, X. I. P. Hernandez, A. DeLaRiva, M. Wang, M. H. Engelhard, L. Kovarik, A. K. Datye, Y. Wang, Science 2017, 358, 1419.

Q. Liu, Z. Zhang, Catal. Sci. Technol. 2019, 9, 4821.

C. D. Powell, A. W. Daigh, M. N. Pollock, B. D. Chandler, C. J. Pursell, J. Phys. Chem. C 2017, 121, 24541.

A. Mahdavi‐Shakib, K. B. S. Kumar, T. N. Whittaker, T. Xie, L. C. Grabow, R. M. Rioux, B. D. Chandler, Angew. Chem. 2021, 133, 7814.

A. Walter, W. Eisenreich, G. Storch, Angew. Chem. 2023, 62, 202310634.

X. Wang, A. Rosspeintner, A. Ziarati, J. Zhao, T. Bürgi, Nat. Commun. 2022, 13, 5458.

A. Corma, P. Serna, P. Concepción, J. J. Calvino, J. Am. Chem. Soc. 2008, 130, 8748.

C. Dessal, A. Sangnier, C. Chizallet, C. Dujardin, F. Morfin, J.‐L. Rousset, M. Aouine, M. Bugnet, P. Afanasiev, L. Piccolo, Nanoscale 2019, 11, 6897.

S. Duan, R. Wang, J. Liu, Nanotechnology 2018, 29, 204002.

Najít záznam

Citační ukazatele

Nahrávání dat ...

Možnosti archivace

Nahrávání dat ...