Injectable materials have shown great potential in tissue engineering applications. However, bacterial infection is one of the main challenges in using these materials in the field of regenerative medicine. In this study, biogenically synthesized silver nanoparticle-decorated multi-walled carbon nanotubes (Ag/MWCNTs) were deployed for adorning biogenic-derived AgNPs which were subsequently used in the preparation of thermosensitive hydrogels based on hyaluronic acid encompassing these green-synthesized NPs. The antibacterial capacity of AgNPs decorated on MWCNTs synthesized through Camellia sinensis extract in an organic solvent-free medium displayed a superior activity by inhibiting the growth of Gram-negative (E. coli and Klebsiella) and Gram-positive (S. aureus and E. faecalis). The injectable hydrogel nanocomposites demonstrated good mechanical properties, as well. The thermosensitive hyaluronic acid-based hydrogels also exhibited Tgel below the body temperature, indicating the transition from liquid-like behavior to elastic gel-like behavior. Such a promising injectable nanocomposite could be applied as liquid, pomade, or ointment to enter wound cavities or bone defects and subsequently its transition in situ to gel form at human body temperature bodes well for their immense potential application in the biomedical sector.

• Keywords
• Ag NPs, Antibacterial, Camellia sinensis, Green synthesis, Injectable nanocomposite, Nanomedicine, Thermosensitive hydrogels,
• Publication type
• Journal Article MeSH

Numerous hazardous environmental pollutants in water bodies, both organic and inorganic, have become a critical global issue. As greener and bio-synthesized versions of nanoparticles exhibit significant promise for wastewater treatment, this review discusses trends and future prospects exploiting the sustainable applications of green-synthesized nanocatalysts and nanomaterials for the removal of contaminants and metal ions from aqueous solutions. Recent trends and challenges about these nanocatalysts and nanomaterials and their potential applications in wastewater treatment and water purification are highlighted including toxicity and biosafety issues. This review delineates the pros and cons and critical issues pertaining to the deployment of these nanomaterials endowed with their superior surface area, mechanical properties, significant chemical reactivity, and cost-effectiveness with low energy consumption, for removal of hazardous materials and contaminants from water; comprehensive coverage of these materials for industrial wastewater remediation, and their recovery is underscored by recent advancements in nanofabrication, encompassing intelligent and smart nanomaterials.

• Keywords
• Biogenic nanomaterials, Green synthesis, Nanocatalysts, Sustainable methods, Water treatment,
• Publication type
• Journal Article MeSH
• Review MeSH