The assembly-disassembly-organization-reassembly (ADOR) process has been used to disassemble a parent zeolite with the UOV structure type and then reassemble the resulting layers into a novel structure, IPC-12. The structure of the material has previously been predicted computationally and confirmed in our experiments using X-ray diffraction and atomic resolution STEM-HAADF electron microscopy. This is the first successful application of the ADOR process to a material with porous layers.

Advanced Microscopy Laboratory University of Zaragoza Mariano Esquillor Edificio 1 D Zaragoza 50018 Spain

Department of Physical and Macromolecular Chemistry Faculty of Science Charles University Hlavova 8 128 43 Prague 2 Czech Republic

Institute of Organic Chemistry and Biochemistry Academy of Sciences of the Czech Republic v v i Flemingovo nám 2 16610 Prague Czech Republic

J Heyrovský Institute of Physical Chemistry Academy of Sciences of the Czech Republic v v i Dolejškova 3 182 23 Prague 8 Czech Republic

School of Chemistry University of St Andrews Purdie Building St Andrews KY16 9ST UK

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ADOR zeolite with 12 × 8 × 8-ring pores derived from IWR germanosilicate

Mechanochemically assisted hydrolysis in the ADOR process

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In situ solid-state NMR and XRD studies of the ADOR process and the unusual structure of zeolite IPC-6